pH-Sensitive CNC-Chitosan Hydrogel for Drug Delivery

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Felycia Edi Soetaredjo, Suryadi Ismadji, Shella Permatasari Santoso, Jindrayani Nyoo Putro, Kuncoro Foe, Gladdy L. Waworuntu

2024 Letters in Applied NanoBioScience Vol. 13 Issue 4 Article Cited by 5 Quartile

Abstract

In contemporary society, inflammatory bowel disease (IBD) is prevalent and acknowledged. In treating inflammatory bowel disease (IBD), pH-sensitive drug delivery systems are commonly utilized. Nonetheless, their efficacy tends to be reduced as a result of modifications in the pH levels within the intestines. This study aims to develop a medication delivery system responsive to changes in pH to deliver 5-aminosalicylic acid specifically to the colon. CNC-chitosan hydrogel was produced by implementing the cross-linking technique, employing glutaraldehyde as the cross-linking agent. The hydrogel was subjected to characterization using scanning electron microscopy (SEM), X-ray diffraction (XRD), swelling capacity analysis, and Fourier-transform infrared spectroscopy (FTIR). The release kinetics of 5-aminosalicylic acid from cellulose nanocrystals (CNC) and CNC-chitosan composites showed superior performance at pH 7.4 compared to pH 2.4. The release profile of 5-aminosalicylic acid from CNC-chitosan hydrogel can be accurately represented by the Korsemeyar-Peppas equation. CNC and CNC-chitosan were compatible with osteoblast cells, indicating their lack of toxicity. © 2024 by the authors.

Affiliations

Department of Chemical Engineering, Widya Mandala Surabaya Catholic University, Indonesia; Collaborative Research Center for Zero Waste and Sustainability, Jl. Kalijudan 37, East Java, Surabaya, 60114, Indonesia; Faculty of Pharmacy, Widya Mandala Surabaya Catholic University, Kalisari Selatan No.1 Kalisari, Surabaya, 60112, Indonesia; Faculty of Medicine, Widya Mandala Surabaya Catholic University, Kalisari Selatan No.1 Kalisari, Surabaya, 60112, Indonesia